You have to realize that all teh files already in your system, including all the system files that make up an "installation," exist already on a given file system. Changing the file system in situ would probably mean creating zfs partitions, transfering files from old partition to new, deleting old partition, and so on. I can't imagine this wouldn't be almost guaranteed to break everything.
Instead, if you are able, it might be advisable to create a backup of all your personal and configuration files, ideally in a device formatted for zfs, and then perform a clean zfs-on-root install on your system.